The truck has been parked since the post above until recently. (3 years plus the one year since I started on the repair) Having my other Tahoe stolen (that's another story) forced me into fixing this one.
What happened up to this point and my attempts at repair compounded the situation and made diagnosis all but impossible with the limited experience I have on these vehicles (and I'm an old school auto technician and currently a master electrician).
So I had it towed to an independent one man shop which I became acquainted with when getting into this originally.
Ultimately the main issue was traced to the throttle body wiring harness. More specifically, to the ground wire in that harness that connected to the passenger side cylinder head.
I had complicated matters by: removing and re-installing the (same) PCM, replacing the electrical side of the ignition switch and as it turns out trying to do my troubleshooting (via a Tech 2) with a faulty (truck) battery.
Interestingly, it was this battery that led to the original no start condition that arose after having been parked for two weeks. The intermittent electrical was already an issue prior to this. The battery in question showed proper voltage. It also load tested well. It was off and on various chargers (smart and otherwise). What the battery was doing was performing as it normally would then for whatever reason, (perhaps via an internal short) would sort of half drop out. When this happened, the instrument cluster would not fully shut down, the door locks became inoperable and the ignition switch lost most of it's functionality. There were probably other issues as well but the gauges not shutting down entirely would ultimately drain the battery over a day. I never got to the point of starting from square one again as another truck purchase put this on the back burner. It was my mechanic who related this same story to me and it fit perfectly with what I had experienced in my testing. Various batteries had been in and out but as it happened, the faulty battery was in the truck when it arrived at the shop.
Anyway, to sum it up, the original intermittent electrical was traced to a poor ground and the inability to diagnose this (as the Tech 2 kept losing communication) was traced to the battery.
The truck is now back in service.